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Synthesis and antibacterial evaluation of calcinated Ag-doped nano-hydroxyapatite with dispersibility

Abstract

Purpose

Dispersible hydroxyapatite (HAp) nanoparticles are very useful for applying a monolayer to implantable medical devices using the nano-coating technique. To improve tolerance to infection on implanted medical devices, silver-doped HAp (Ag-HAp) nanoparticles with dispersiblity and crystallinity were synthesized, avoiding calcination-induced sintering, and evaluated for antibacterial activity.

Methods

The Ca10-xAgx(PO4)6(OH)2 with x = 0 and 0.2 were prepared by wet chemical processing at 100°C. Before calcination at 700°C for 2 h, two kinds of anti-sintering agents, namely a Ca(NO3)2 (Ca salt) and a polyacrylic acid/Ca salt mixture (PAA-Ca), were used. Escherichia coli was used to evaluate the antibacterial activity of the nanopowder.

Results

When PAA-Ca was used as an anti-sintering agent in calcination to prepare the dispersible nanoparticles, strong metallic Ag peaks were observed at 38.1° and 44.3° (2θ) in the X-ray diffraction (XRD) profile. However, the Ag peak was barely observed when Ca salt was used alone as the anti-sintering agent. Thus, using Ca salt alone was more effective for preparation of dispersible Ag-HAp than PAA-Ca. The particle average size of Ag-HAp with 0.5 mol% of Ag content was found to be 325 ± 70 nm when the formation of large particle-aggregations was prevented, as determined by dynamic light scattering instrument. The antibacterial activity of the Ag-HAp nanoparticles possessing 0.5 mol% against E. coli was greater than 90.0%.

Conclusions

Dispersible and crystalline nano Ag-HAp can be obtained by using Ca salt alone as an anti-sintering agent. The nanoparticles showed antibacterial activity.

Int J Artif Organs 2015; 38(5): 251 - 258

Article Type: ORIGINAL RESEARCH ARTICLE

DOI:10.5301/ijao.5000408

Authors

Tsutomu Furuzono, Mazumder Motaharul, Yasumichi Kogai, Yoshinao Azuma, Yoshiki Sawa

Article History

Disclosures

Financial support: The study was supported in a part by JSPS Grant-in-Aid for Scientific Research (C) (KAKENHI), grant number 25350557, and a grant from the MEXT-Supported Program for the Strategic Research Foundation at Private Universities, grant number S1311045.
Conflict of Interest: T. Furuzono serves as a consultant to SofSera Corporation.

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Authors

  • Furuzono, Tsutomu [PubMed] [Google Scholar] 1, 2, * Corresponding Author ([email protected])
  • Motaharul, Mazumder [PubMed] [Google Scholar] 1, 3
  • Kogai, Yasumichi [PubMed] [Google Scholar] 3
  • Azuma, Yoshinao [PubMed] [Google Scholar] 4
  • Sawa, Yoshiki [PubMed] [Google Scholar] 2

Affiliations

  • Department of Biomaterial Engineering, School of Biology-Oriented Science and Technology, Kinki University, Wakayama - Japan
  • Department of Surgery, Osaka University Graduate School of Medicine, Osaka - Japan
  • Technical Development Center, SofSera Corporation, Osaka - Japan
  • Department of Science and Technology on Food Safety, School of Biology-Oriented Science and Technology, Kinki University, Wakayama - Japan

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